John Williams scored episodes: "Officer's Mess" 9/8/1966 "How to Steal a Girl Even If It's Only Me" 9/15/1966 "Tammy Takes Las Vegas, or Vice Versa" 9/22/1966 "Positively Made in Paris" 9/29/1966
These episodes never aired but may have contained music by Williams: "George Washington Didn't Sleep Here" "Send a Rich Girl to Camp This Summer" "Tammy Plays Cupid" "A Funny Thing Happened to Me on the Way to the Studio" "Tamantha Nightingale Rides Again" "Diamonds Are a Bird's Best Friend"
Tammy Grimes spent most of her acting/singing career in television and on stage. She won a 1960 Tony award for her title role in "The Unsinkable Molly Brown" on Broadway. She had major roles in only a handful of films, the first of which was:
According to the Williams buyer's guide in FSM (which I often use for reference), he wrote 2-3 episode scores as well. Well, he didn't write the one that's available on youtube, so it must be the others then (or some of the unaired ones).